By M. Ya. Amusia (auth.), Uwe Becker, David A. Shirley (eds.)
Leading investigators supply the 1st entire examine of fuel part photoionization study within the VUV and delicate X-ray regime because the huge employment of synchrotron radiation as a spectroscopic instrument. Chapters hide all facets of photoionization phenomena from overall pass sections to hugely differentiated measurements reminiscent of accident experiments and spin-resolved electron spectroscopy. This paintings is plentiful with illustrations.
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Additional info for VUV and Soft X-Ray Photoionization
4d 0) . 4d ~ ;-'-~: (50) E At fIrst glance it is a surprise that a highly excited electron can affect the inner vacancy decay. However, the 4d electron, being loosely bound, can easily change its state due to the alteration of the field acting on this electron after Auger decay. Indeed, it appeared that the overlap integral (4d 14d) is nearly zero and most probable is the decay of the 2p vacancy accompanied by the 4d electron traMitions to higher excited level~5d, 6d, and some others. Thus, the total decay probability is not altered, while the intensities of its particular channels are redistributed.
I' which can be estimated as (45) VI being the slow photoelectron's speed. In (45) rjA) is the Auger width of the vacancy i. A»II2. I It is easy to take into account the interaction of two outgoing electrons 61 and ~ with velocities and V2 semic1assically, having in mind that the distance between them after the period of decay (r~A~-1 is IV2 -VI I ;r~A) . This modifies the expression (45) leading to v) (46) It is seen from (46), according to what was demonstrated in Ref. ,£j for rapidly decaying vacancies, although the relative value Ae/ri decreases with r j growth.
It is essential to have in mind that static rearrangement corresponds only to parts ofthese diagrams even in the order considered of the perturbation in the interelectron interaction theory: instead of a summation over all intermediate vacancy states, only the term with the vacancy i is taken into account. By including in the RPAE scheme the corrections of the type discussed, the generalized RPAE (GRPAE) is fonned. F (15) 17 THEORY OF PHOTOJONIZATION Here the sign - under an electron or vacancy wave function emphasizes that these states are calculated in the HF field of an ion with a vacancy, namely, a state (~,i) in the presence of the vacancy i and (~,i') in the presence of the vacancy r.
VUV and Soft X-Ray Photoionization by M. Ya. Amusia (auth.), Uwe Becker, David A. Shirley (eds.)